A long-term goal for superconductors is to increase the superconducting transition temperature, T-C. In cuprates, T-C depends strongly on the out-of-plane Cu-apical oxygen distance and the in-plane Cu-O distance, but there has been little attention paid to tuning them independently. Here, in simply grown, self-assembled, vertically aligned nanocomposite thin films of La2CuO4+delta + LaCuO3, by strongly increasing out-of-plane distances without reducing in-plane distances (three-dimensional strain engineering), we achieve superconductivity up to 50 K in the vertical interface regions, spaced similar to 50 nm apart. No additional process to supply excess oxygen, e.g., by ozone or high-pressure oxygen annealing, was required, as is normally the case for plain La2CuO4+delta. films. Our proof-of-concept work represents an entirely new approach to increasing T-C in cuprates or other superconductors.

3D strain-induced superconductivity in La2CuO4+δ using a simple vertically aligned nanocomposite approach

Di Bernardo, Angelo;
2019-01-01

Abstract

A long-term goal for superconductors is to increase the superconducting transition temperature, T-C. In cuprates, T-C depends strongly on the out-of-plane Cu-apical oxygen distance and the in-plane Cu-O distance, but there has been little attention paid to tuning them independently. Here, in simply grown, self-assembled, vertically aligned nanocomposite thin films of La2CuO4+delta + LaCuO3, by strongly increasing out-of-plane distances without reducing in-plane distances (three-dimensional strain engineering), we achieve superconductivity up to 50 K in the vertical interface regions, spaced similar to 50 nm apart. No additional process to supply excess oxygen, e.g., by ozone or high-pressure oxygen annealing, was required, as is normally the case for plain La2CuO4+delta. films. Our proof-of-concept work represents an entirely new approach to increasing T-C in cuprates or other superconductors.
2019
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Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/11386/4825814
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